The first album: Begin Here (1965)
Danger Man, season 3, episode 3, "Sting in the Tail" (1965): soundtrack features Jeanne Roland singing the French adaptation of "She's Not There", "Te voila", in background and occasionally foreground (since the time cuts are weirdly resistant to being saved--when they don't insert themselves--on Blogspot, at 17:00 is a good point to start the relevant performance; a bit of it used in reprise at end of [a very good] episode):
The Zombies on a pub tv: "Just Out of Reach" and "Nothing's Changed"
Odessey and Oracle the album (1968)
"Ma Non E Giusto" ("She's Not There" in Italian)